湖北泉水河流域水化学特征和硝酸盐来源示踪

李严; 曹明达; 靳孟贵; 张结; 黄鑫

doi:10.3799/dqkx.2019.060

Volume 45 Issue 3

Mar. 2020

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Li Yan, Cao Mingda, Jin Menggui, Zhang Jie, Huang Xin, 2020. Hydrochemical Characteristics and Tracing of Nitrate Sources in Quanshui River Catchment, Hubei Province. Earth Science, 45(3): 1061-1070. doi: 10.3799/dqkx.2019.060

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Li Yan, Cao Mingda, Jin Menggui, Zhang Jie, Huang Xin, 2020. Hydrochemical Characteristics and Tracing of Nitrate Sources in Quanshui River Catchment, Hubei Province. Earth Science, 45(3): 1061-1070. doi: 10.3799/dqkx.2019.060

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Hydrochemical Characteristics and Tracing of Nitrate Sources in Quanshui River Catchment, Hubei Province

doi: 10.3799/dqkx.2019.060

Li Yan^{1,2
,
,},
Cao Mingda^1,2,
Jin Menggui^{1,2
,
,
,},
Zhang Jie^1,2,
Huang Xin^1,2

1.
Laboratory of Basin Hydrology and Wetland Eco-Restoration, China University of Geosciences, Wuhan 430074, China
2.
School of Environmental Studies, China University of Geosciences, Wuhan 430074, China

Received Date: 2019-02-13
Publish Date: 2020-03-15

Abstract

Abstract

There are few studies on the source identification of nitrate in the natural rivers in karst area, and even fewer on the influence of the anti-seasonal arid climate on the nitrate transportation. In this paper, δ¹⁵N and δ¹⁸O isotopic tracing method is used to analyze the source of nitrate in surface water and groundwater of Quanshui River, a branch of Hangjiang River and to determine the biological and chemical transformation process of nitrate. The contribution rate of each pollution terminal element was determined quantitatively by using the model of Stable Isotope Analysis in R (SIAR). The results show that soil organic nitrogen, sewage manure, fertilizer and atmospheric subsidence contributed 31.4%, 20.0%, 29.6% and 19.0% respectively to the nitrate source of groundwater, and the proportion of nitrate source to surface water was 32.0%, 30.0%, 25.0% and 13.0%. The contribution of sewage manure to surface water nitrate is significantly higher than that of groundwater. Due to the large water body, the water in the reservoir has strong self-purification ability and is almost unaffected by sewage manure (only 9.0%).The contribution of soil organic nitrogen, atmospheric subsidence and fertilizer in the nitrate soil of the reservoir was 43.0%, 11.0% and 37.0%, respectively. In dry season, groundwater is mainly recharged slowly by groundwater. Because groundwater is affected by soil in vadose zone, soil organic nitrogen is the main source of nitrate in the river. The downstream of the river is more susceptible to human activities, and the contribution of domestic sewage and chemical fertilizer to nitrate in rivers increases.
- nitrate pollution,
- nitrogen and oxygen isotopes,
- source identification,
- SIAR model,
- Quanshui River,
- hydrogeology

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References(43)

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Hydrochemical Characteristics and Tracing of Nitrate Sources in Quanshui River Catchment, Hubei Province

doi: 10.3799/dqkx.2019.060

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