Volume 41 Issue 11
Nov.  2016
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Wang Qianru, Chen Honghan, Hu Shouzhi, Zhao Yutao, Chen Huiqin, 2016. Curve-Fitting Analysis of Micro FT-IR and Its Application on Individual Oil Inclusion and Micro-Area Bitumens. Earth Science, 41(11): 1921-1934. doi: 10.3799/dqkx.2016.133
Citation: Wang Qianru, Chen Honghan, Hu Shouzhi, Zhao Yutao, Chen Huiqin, 2016. Curve-Fitting Analysis of Micro FT-IR and Its Application on Individual Oil Inclusion and Micro-Area Bitumens. Earth Science, 41(11): 1921-1934. doi: 10.3799/dqkx.2016.133
shu

Curve-Fitting Analysis of Micro FT-IR and Its Application on Individual Oil Inclusion and Micro-Area Bitumens

doi: 10.3799/dqkx.2016.133
  • 1.

    Key Laboratory of Tectonics and Petroleum Resources of Ministry of Education, China University of Geosciences, Wuhan 430074, China

  • 2.

    Jilin Oil Field Exploitation Research Institute, PetroChina, Songyuan 138001, China

  • Received Date: 2016-01-10
  • Publish Date: 2016-11-15
    Abstract
  • Curve-fitting analysis of micro FT-IR, in the theory of Gaussian, Lorentz function or their combination (Gaussian-Lorentz) model, can break through the limit of overlapping spectra resulting from complicated structures of samples (e.g. individual oil inclusion and bitumens). Hence, curve-fitting analysis of micro FT-IR was used for analyzing maturity of individual oil inclusion and the origin of bitumens in Shuntuoguole area of Tazhong northeastern slope systematically, and four conclusions have been obtained: firstly, curve-fitting analysis of micro FT-IR may be more accurate for calculating absorption peaks, and some easily neglected peaks can be detected by this method in contrast with the method of interval oriented by Pironon. Secondly, Gaussian-Lorentz fitting is more approaching to actual spectra and the lower noise level is corresponding to better fit but requiring longer computation time. As a result, Gaussian-Lorentz fitting with 1~10 noise level is preferred. Thirdly, based on inclusion system analysis and burial history projection with homogenization temperature, infrared parameters (e.g. CH2a/CH3a, Xinc and Xstd) reveal three hydrocarbon charging events occurred, including Late Caledonian, Late Hercynian and the Himalaya. Finally, micro FT-IR is an effective means for analyzing multi-hydrocarbon charging events and complicated origin of bitumens undergoing biodegradation, oxidative degradation and water eluviation quantitatively in study area.

     

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  • Adebiyi, F.M., Odunlami, A., Thoss, V., 2015.Chemical Studies of High Molecular Weight Fractions of Nigerian Bitumen.Journal of Unconventional Oil and Gas Resources, 9:84-93.doi: 10.1016/j.juogr.2014.11.002
    Carbognani, L., Orea, M., Fonseca, M., 1999.Complex Nature of Separated Solid Phases from Crude Oils.Energy & Fuels, 13(2):351-358.doi: 10.1021/ef9801975
    Chen, Y., Mastalerz, M., Schimmelmann, A., 2012.Characterization of Chemical Functional Groups in Macerals Across Different Coal Ranks Via Micro-FTIR Spectroscopy.International Journal of Coal Geology, 104:22-33.doi: 10.1016/j.coal.2012.09.001
    Domke, C.H., Davison, R.R., Glover, C.J., 1999.Effect of Asphaltenes on SHRP Superpave Specifications.Energy & Fuels, 13(2):340-345.doi: 10.1021/ef980194s
    Fan, X.Y., Wu, X.L., Meng, D.W., et al., 2007.Water in UHP Jadeite-Quartzites of Dabie Mountains: Evidence from Micro-FTIR.Earth Science, 32(2):167-174 (in Chinese with English abstract). http://en.cnki.com.cn/article_en/cjfdtotal-dqkx200702002.htm
    Ferket, H., Guilhaumou, N., Roure, F., et al., 2011.Insights from Fluid Inclusions, Thermal and PVT Modeling for Paleo-Burial and Thermal Reconstruction of the Córdoba Petroleum System (NE Mexico).Marine and Petroleum Geology, 28(4):936-958.doi: 10.1016/j.marpetgeo.2010.01.020
    Fu, M.Y., Liu, F., Deng, H.C., et al., 2015.Hydrocarbon Charging Period of Cretaceous Reservoirs in AHDEB Oil Field:Evidence from Fluid Inclusions.Earth Science, 40(7):1187-1196(in Chinese with English abstract). http://en.cnki.com.cn/Article_en/CJFDTotal-DQKX201507007.htm
    Ganz, H., Kalkreuth, W., 1987.Application of Infrared Spectroscopy to the Classification of Kerogen Types and the Evaluation of Source Rock and Oil Shale Potentials.Fuel, 66(5):708-711.doi: 10.1016/0016-2361(87)90285-7
    George, S.C., Llorca, S.M., Hamilton, P.J., 1994.An Integrated Analytical Approach for Determining the Origin of Solid Bitumens in the McArthur Basin, Northern Australia.Organic Geochemistry, 21(3-4):235-248.doi: 10.1016/0146-6380(94)90187-2
    Goodarzi, F., Williams, P.F.V., 1986.Composition of Natural Bitumens and Asphalts from Iran:2.Bitumens from the Posteh Ghear Valley, South-West Iran.Fuel, 65(1):17-27.doi: 10.1016/0016-2361(86)90136-5
    Gui, L.L., Liu, K.Y., Liu, S.B., et al., 2015.Hydrocarbon Charge History of Yingdong Oilfield, Western Qaidam Basin.Earth Science, 40(5):890-899 (in Chinese with English abstract). https://www.researchgate.net/publication/282059958_Hydrocarbon_charge_history_of_Yingdong_Oilfield_Western_Qaidam_Basin
    Han, F., Zhang, Y.G., Meng, A.H., et al., 2014.FTIR Analysis of Yunnan Lignite.Journal of China Coal Society, 39(11):2293-2299(in Chinese with English abstract). http://en.cnki.com.cn/Article_en/CJFDTotal-MTXB201411024.htm
    Hu, Y.G., Zhang, X.X., Zhao, Z.Y., et al., 2012.Strategy and Implementation of Resolve Overlapping Spectra Based on Curve Fitting.Journal of Chongqing University, 35(5):76-82(in Chinese with English abstract). http://en.cnki.com.cn/Article_en/CJFDTOTAL-FIVE201205012.htm
    Ignasiak, T., Kemp-Jones, A.V., Strausz, O.P., 1977.The Molecular Structure of Athabasca Asphaltene.Cleavage of the Carbon-Sulfur Bonds by Radical Ion Electron Transfer Reactions.The Journal of Organic Chemistry, 42(2):312-320.doi: 10.1021/jo00422a031
    Karakaplan, M., 2007.Fitting Lorentzian Peaks with Evolutionary Genetic Algorithm Based on Stochastic Search Procedure.Analytica Chimica Acta, 587(2):235-239.doi: 10.1016/j.aca.2007.01.058
    Khorasani, G.K., 1987.Novel Development in Fluorescence Microscopy of Complex Organic Mixtures:Application in Petroleum Geochemistry.Organic Geochemistry, 11(3):157-168.doi: 10.1016/0146-6380(87)90019-2
    Kim, D., Philp, R.P., Sorenson, R.P., 2010.Geochemical Characterization of Solid Bitumen in the Chesterian (Mississippian) Sandstone Reservoir of the Hitch Field, Southwest Kansas.AAPG Bulletin, 94(7):1031-1057.doi: 10.1306/12090909096
    Kuehn, D.W., Snyder, R.W., Davis, A., et al., 1982.Characterization of Vitrinite Concentrates.1.Fourier Transform Infrared Studies.Fuel, 61(8):682-694.doi: 10.1016/0016-2361(82)90240-x
    Landais, P., 1995.Statistical Determination of Geochemical Parameters of Coal and Kerogen Macerals from Transmission Micro-Infrared Spectroscopy Data.Organic Geochemistry, 23(8):711-720.doi: 10.1016/0146-6380(95)00070-u
    Li, W.G., Duan, Y.H., Yan, L.K., et al., 2012.Study on Measuring Method of Asphalt Using Infrared Spectrum Characteristic of Petroleum Pitch.Petroleum Asphalt, 26(4):9-14(in Chinese with English abstract). http://en.cnki.com.cn/Article_en/CJFDTOTAL-OILE201204006.htm
    Lis, G.P., Mastalerz, M., Schimmelmann, A., et al., 2005.FTIR Absorption Indices for Thermal Maturity in Comparison with Vitrinite Reflectance R0 in Type-Ⅱ Kerogens from Devonian Black Shales.Organic Geochemistry, 36(11):1533-1552.doi: 10.1016/j.orggeochem.2005.07.001
    Liu, D.M., Jin, K.L., Wang, L.Z., 1999.Characteristics and Genesis of Silurian Bituminous Sandstone in the Tarim Basin.Geoscience, 13(2):169-175(in Chinese with English abstract). http://en.cnki.com.cn/Article_en/CJFDTOTAL-XDDZ902.008.htm
    Liu, D.M., Yang, Q., Tang, D.Z., 1998.Micro-FTIR Analysis of Macerals in Coals from the Ordos Basin.Earth Science, 23(1):79-84(in Chinese with English abstract). http://en.cnki.com.cn/Article_en/CJFDTotal-DQKX801.017.htm
    Liu, L.F., Zhao, J.Z., Zhang, S.C., et al., 2000.Genetic Types and Characteristics of the Silurian Asphaltic Sandstones in Tarim Basin.Acta Petrolei Sinica, 21(6):12-17 (in Chinese with English abstract). http://www.syxb-cps.com.cn/EN/Y2000/V21/I6/12
    Liu, L.F., Zhao, J.Z., Zhang, S.C., et al., 2001.The Depositional and Structural Settings and the Bituminous Sandstone Distribution Characters of the Silurian in Tarim Basin.Acta Petrolei Sinica, 22(6):11-17 (in Chinese with English abstract). http://en.cnki.com.cn/Article_en/CJFDTOTAL-SYXB200106002.htm
    Liu, Z.F., Colin, C., Trentesaux, A., 2005.Application of Fourier Transform Infrared (FTIR) Spectroscopy in Quantitative.Earth Science, 30(1):25-29 (in Chinese with English abstract). https://zh.scribd.com/document/183374455/Application-of-Fourier-Transform-Infrared-Spectroscopy-FTIR
    Lórenz-Fonfría, V.A., Padrós, E., 2004.Curve-Fitting of Fourier Manipulated Spectra Comprising Apodization, Smoothing, Derivation and Deconvolution.Spectrochimica Acta Part A:Molecular and Biomolecular Spectroscopy, 60(12):2703-2710.doi: 10.1016/j.saa.2004.01.008
    Mastalerz, M., Glikson, M., 2000.In-Situ Analysis of Solid Bitumen in Coal:Examples from the Bowen Basin and the Illinois Basin.International Journal of Coal Geology, 42(2-3):207-220.doi: 10.1016/s0166-5162(99)00040-3
    Nieuwoudt, M.K., Simpson, M.P., Tobin, M., et al., 2014.Synchrotron FTIR Microscopy of Synthetic and Natural CO2-H2O Fluid Inclusions.Vibrational Spectroscopy, 75:136-148.doi: 10.1016/j.vibspec.2014.08.003
    Okolo, G.N., Neomagus, H.W.J.P., Everson, R.C., et al., 2015.Chemical-Structural Properties of South African Bituminous Coals:Insights from Wide Angle XRD-Carbon Fraction Analysis, ATR-FTIR, Solid State 13C NMR, and HRTEM Techniques.Fuel, 158:779-792.doi: 10.1016/j.fuel.2015.06.027
    Painter, P.C., Snyder, R.W., Starsinic, M., et al., 1981.Concerning the Application of FT-IR to the Study of Coal:A Critical Assessment of Band Assignments and the Application of Spectral Analysis Programs.Applied Spectroscopy, 35(5):475-485.doi: 10.1366/0003702814732256
    Parente, M., Makarewicz, H.D., Bishop, J.L., 2011.Decomposition of Mineral Absorption Bands Using Nonlinear Least Squares Curve Fitting:Application to Martian Meteorites and CRISM Data.Planetary and Space Science, 59(5-6):423-442.doi: 10.1016/j.pss.2011.01.009
    Pironon, J., Barres, O., 1990.Semi-Quantitative FT-IR Microanalysis Limits:Evidence from Synthetic Hydrocarbon Fluid Inclusions in Sylvite.Geochimica et Cosmochimica Acta, 54(3):509-518.doi: 10.1016/0016-7037(90)90348-o
    Pironon, J., Thiéry, R., Teinturier, S., et al., 2000.Water in Petroleum Inclusions:Evidence from Raman and FT-IR Measurements, PVT Consequences.Journal of Geochemical Exploration, 69-70:663-668.doi: 10.1016/s0375-6742(00)00108-4
    Qin, Z.H., Chen, H., Yan, Y.J., et al., 2015.FTIR Quantitative Analysis Upon Solubility of Carbon Disulfide/N-Methyl-2-Pyrrolidinone Mixed Solvent to Coal Petrographic Constituents.Fuel Processing Technology, 133:14-19.doi: 10.1016/j.fuproc.2015.01.001
    Sobkowiak, M., Painter, P., 1992.Determination of the Aliphatic and Aromatic CH Contents of Coals by FT-I.R.:Studies of Coal Extracts.Fuel, 71(10):1105-1125.doi: 10.1016/0016-2361(92)90092-3
    Strausz, O.P., Mojelsky, T.W., Faraji, F., et al., 1999.Additional Structural Details on Athabasca Asphaltene and their Ramifications.Energy & Fuels, 13(2):207-227.doi: 10.1021/ef980274w
    Walters, C.C., Qian, K.N., Wu, C.P., et al., 2011.Proto-Solid Bitumen in Petroleum Altered by Thermochemical Sulfate Reduction.Organic Geochemistry, 42(9):999-1006.doi: 10.1016/j.orggeochem.2011.08.001
    Wang, C.J., Cao, D.Y., Chen, J.M., et al., 2014.Formation Mechanism of Aggregated Type Natural Bitumen with High Evolution Degree:With Vein Anthraxolite in Xiangxi as an Instance.Science & Technology Review, 32(24):40-45. http://en.cnki.com.cn/Article_en/CJFDTotal-KJDB201424018.htm
    Wang, Q.J., Chen, J.Y., 1988.Petroleum Geochemistry.China University of Geosciences Press, Wuhan, 220-224(in Chinese).
    Weng, S.F, 2010.Fourier Transform Infrared Spectrum Analysis.Chemical Industry Press, Beijing, 269-272 (in Chinese).
    Wilhelms, A., Larter, S.R., 1994.Origin of Tar Mats in Petroleum Reservoirs.Part Ⅰ:Introduction and Case Studies.Marine and Petroleum Geology, 11(4):418-441.doi: 10.1016/0264-8172(94)90077-9
    Xiong, G., Li, Y.S., Jin, L.J., et al., 2015.In-Situ FT-IR Spectroscopic Studies on Thermal Decomposition of the Weak Covalent Bonds of Brown Coal.Journal of Analytical and Applied Pyrolysis, (115):262-267.doi: 10.1016/j.jaap.2015.08.002
    Xu, L., Liu, F., Shen, B.X., et al., 2011.Characterization of Tahe Asphalt.Science & Technology in Chemical Industry, 19(4):44-46(in Chinese with English abstract). http://en.cnki.com.cn/Article_en/CJFDTotal-JKGH201104012.htm
    Xu, W., Liu, X.W., Jin, Z.M., 2006.Water in UHP Eclogites at CCSD:FTIR Analysis.Earth Science, 31(6):830-838(in Chinese with English abstract). http://en.cnki.com.cn/Article_en/CJFDTOTAL-DQKX200606011.htm
    Zhang, J.H., Liu, Q., Chen, Y.M., et al., 2012.Determination of Acid Dissociation Constant of Methyl Red by Multi-Peaks Gaussian Fitting Method Based on UV-Visible Absorption Spectrum.Acta Physico-Chimica Sinica, 28(5):1030-1036. http://en.cnki.com.cn/Article_en/CJFDTOTAL-WLHX201205005.htm
    Zhang, J., Pang, X.Q., Liu, L.F., et al., 2004.Distribution Characteristics and Petroleum Gesignificance of the Silurian Asphaltic Sandstones in Tarim Basin.Science in China (Series D), 47(S2):199-208(in Chinese).doi: 10.1360/04zd0039
    Zou, Y.L., Yu, X., Li, S.H., et al., 2005.Study on Hydrocarbon Reservoir Formation Period Using Microscope-Infrared Spectroscopy Method.Petroleum Geology & Oilfield Development in Daqing, 24(03):33-34 (in Chinese with English abstract). http://en.cnki.com.cn/Article_en/CJFDTOTAL-DQSK200503014.htm
    樊孝玉, 吴秀玲, 孟大维, 等, 2007.大别山超高压硬玉石英岩中的水:来自红外光谱的证据.地球科学, 32(2):167-174. http://earth-science.net/WebPage/Article.aspx?id=3436
    伏美燕, 刘榧, 邓虎成, 等, 2015.AHDEB油田白垩系油藏油气充注期次的流体包裹体证据.地球科学, 40(7):1187-1196. http://earth-science.net/WebPage/Article.aspx?id=3110
    桂丽黎, 刘可禹, 柳少波, 等, 2015.柴达木盆地西部英东地区油气成藏过程.地球科学, 40(5):890-899. http://earth-science.net/WebPage/Article.aspx?id=3081
    韩峰, 张衍国, 蒙爱红, 等, 2014.云南褐煤结构的FTIR分析.煤炭学报, 39(11):2293-2299. http://www.cnki.com.cn/Article/CJFDTOTAL-MTXB201411024.htm
    胡耀垓, 张晓星, 赵正予, 等, 2012.光谱重叠峰的曲线拟合解析策略与实现.重庆大学学报:自然科学版, 35(5):76-82. http://www.cnki.com.cn/Article/CJFDTOTAL-FIVE201205012.htm
    李炜光, 段炎红, 颜录科, 等, 2012.利用石油沥青红外光谱图谱特征测定沥青的方法研究.石油沥青, 26(4):9-14. http://www.cnki.com.cn/Article/CJFDTOTAL-OILE201204006.htm
    刘大锰, 金奎励, 王凌志, 1999.塔里木盆地志留系沥青砂岩的特性及其成因.现代地质, 13(2):169-175. http://www.cnki.com.cn/Article/CJFDTOTAL-XDDZ902.008.htm
    刘大锰, 杨起, 汤达祯, 1998.鄂尔多斯盆地煤显微组分的micro-FTIR研究.地球科学, 23(1):79-84. http://earth-science.net/WebPage/Article.aspx?id=588
    刘洛夫, 赵建章, 张水昌, 等, 2000.塔里木盆地志留系沥青砂岩的成因类型及特征.石油学报, 21(6):12-17. doi: 10.7623/syxb200006002
    刘洛夫, 赵建章, 张水昌, 等, 2001.塔里木盆地志留系沉积构造及沥青砂岩的特征.石油学报, 22(6):11-17. doi: 10.7623/syxb200106003
    刘志飞, Christophe, C., Alain, T., 2005.傅里叶变换红外光谱(FTIR)方法在南海定量矿物学研究中的应用:以MD01-2393孔为例.地球科学, 30(1):25-29. http://earth-science.net/WebPage/Article.aspx?id=1449
    王崇敬, 曹代勇, 陈健明, 等, 2014.聚集型高演化天然固体沥青成因——以湘西脉状碳沥青为例.科技导报, 32(24):40-45. doi: 10.3981/j.issn.1000-7857.2014.24.005
    王启军, 陈建渝, 1988.油气地球化学.武汉:中国地质大学出版社, 220-224.
    翁诗甫, 2010.傅里叶变换红外光谱分析.北京:化学工业出版社, 269-272.
    徐力, 刘峰, 沈本贤, 等, 2011.塔河沥青表征研究.化工科技, 19(4):44-46. http://www.cnki.com.cn/Article/CJFDTOTAL-JKGH201104012.htm
    徐薇, 刘祥文, 金振民, 2006.CCSD超高压榴辉岩中的水:红外光谱分析.地球科学, 31(6):830-838. http://earth-science.net/WebPage/Article.aspx?id=1646
    张建华, 刘琼, 陈玉苗, 等, 2012.紫外-可见吸收光谱结合高斯多峰拟合技术测定甲基红酸离解常数(英文).物理化学学报, 28(5):1030-1036. http://www.cnki.com.cn/Article/CJFDTOTAL-WLHX201205005.htm
    张俊, 庞雄奇, 刘洛夫, 等, 2004.塔里木盆地志留系沥青砂岩的分布特征与石油地质意义.中国科学(D辑), 34(增刊1):169-176. http://www.cnki.com.cn/Article/CJFDTOTAL-JDXK2004S1019.htm
    邹育良, 俞萱, 李松花, 等, 2005.利用显微-红外光谱法研究油气成藏期次.大庆石油地质与开发, 24(3):33-34. http://www.cnki.com.cn/Article/CJFDTOTAL-DQSK200503014.htm
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